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Citation - WoS: 8
Citation - Scopus: 8
Analysis of the Specific Heat and the Free Energy of [N(ch3)4]2znbr4 Close To the Ferro-Paraelastic Phase Transition
(Taylor & Francis Ltd, 2019) Kiraci, A.; 42475; 09.01. Ortak Dersler Bölümü; 09. Rektörlük; 01. Çankaya Üniversitesi
A power-law formula deduced from the Ising model was used to analyze the temperature dependence of the specific heat and the Gibbs free energy of [N(CH3)(4)](2)ZnBr4 compound in the vicinity of the phase transition temperature of T-C = 287.2 K. Obtained values of the critical exponents from the Gibbs free energy were consistent with that predicted from 2-d potts model ( = 0.3), while obtained values of from the specific heat in both ferroelastic and paraelastic phases were consistent with that predicted from the mean field theory ( = 0) in the vicinity of the phase transition temperature. This is an indication of that [N(CH3)(4)](2)ZnBr4 compound undergoes a second order type phase transition. Also, the enthalpy () and the entropy () of this crystal were calculated in terms of the extracted values of the critical exponent in both ferroelastic and paraelastic phases.
Citation - Scopus: 1
Phenomenological Approaches on the Nd³⁺ Doped Ferroelectric Labgeo5
(Taylor & Francis Ltd, 2021) Kiraci, A.; Yurtseven, Hamit; Kara, N.; 09.01. Ortak Dersler Bölümü; 09. Rektörlük; 01. Çankaya Üniversitesi
Two phenomenological models, namely the compressible Ising model and Landau model, have been used to analyze the specific heat and the dielectric constant data, respectively for the pure and Nd3+ doped LaBGeO5 (LBG) crystals. The critical exponent of the specific heat was extracted in both ferroelectric and paraelectric phases of the crystals studied here within the temperature intervals of [T - T-C vertical bar < 4 K. The extracted values of the critical exponent were then used to predict some thermodynamic quantities such as the enthalpy, entropy, and the Gibbs free energy. Regarding the analysis of dielectric constant data within the framework of the Landau theory, the observed values of the birefringence were associated with the order parameter below the transition temperature T-c. The Landau coefficients a(0) and a(4) were determined. Our results indicate a second-order phase transition mechanism.
Citation - WoS: 2
Citation - Scopus: 2
Phenomenological Study of Manganese Antimonite Close To the Neel Temperature
(Ieee-inst Electrical Electronics Engineers inc, 2021) Kiraci, Ali; 09.01. Ortak Dersler Bölümü; 09. Rektörlük; 01. Çankaya Üniversitesi
The anomalous behavior of the frequency f and specific heat C-p data for the new layered trigonal (P (3) over bar 1m) form of manganese antimonite (MnSb2O6) was analyzed by means of the power-law relations with the critical exponent alpha in the vicinity of the Neel temperature of T-N= 8.0 K. While the extracted values of a from both f and C-p below T-N (the same value of 0.06) match exactly the value 1/16 (= 0.06) predicted from the three-dimensional (3-D) Ising model, the extracted value of 0.65 from the C-p data above T-N is much higher than the predicted value of 1/8 (= 0.13) from the 3-D Ising model. As an extension of this work, the temperature dependence of the muon-spin relaxation rate (damping constant) lambda of MnSb2O6 was calculated from the pseudospin-phonon-coupled (PS) model and the energy fluctuation (EF) model below T-N. Our results are in good agreement with the data. In addition, the activation energy was calculated from the predicted values of. from both PS and EF models for MnSb2O6. Our results indicate an order-disorder-type transition at T-N = 8.0 K for MnSb2O6.
Citation - WoS: 3
Citation - Scopus: 3
A Phenomenological Study on Ferroelastic Kh3(Seo3)2 and Kd3(Seo3)2
(Pergamon-elsevier Science Ltd, 2021) Kiraci, A.; 42475; 09.01. Ortak Dersler Bölümü; 09. Rektörlük; 01. Çankaya Üniversitesi
The anomalous behavior of the Brillouin frequency shift omega of the soft acoustic mode for KH3(SeO3)(2) and KD3(SeO3)(2), and also the volume thermal expansion proportional to(V) and the specific heat C of KH3(SeO3)(2) have been analyzed for various temperature intervals close to the phase transition temperatures TC at around 211 K and 302 K, respectively. Our extracted values of the critical exponent from C and proportional to(V) of KH3(SeO3)(2) within the temperature intervals of vertical bar T -T-C vertical bar < 7 K are nearly zero, while the critical exponent extracted from the Brillouin frequency shift data of both KH3(SeO3)(2) and KD3(SeO3)(2) within the same temperature interval of vertical bar T -T-C vertical bar < 7 K decrease very rapidly toward to zero as the phase transition temperatures are approached. Our results indicate that the critical behavior of omega, proportional to(V) and C of both KH3(SeO3)(2) and KD3(SeO3)(2) can be described with the same critical exponent within the temperature interval of vertical bar T -T-C vertical bar < 2 K.
Citation - WoS: 2
Citation - Scopus: 3
A Phenomenological Study on Ferroelectric Β-Glycine
(Taylor & Francis Ltd, 2021) Kiraci, A.; 42475; 09.01. Ortak Dersler Bölümü; 09. Rektörlük; 01. Çankaya Üniversitesi
The anomalous behavior of the specific heat for beta-glycine was analyzed in terms of the compressible Ising model approximately 5 K below and above the ferrelectric-paraelectric phase transition temperature of T-C =252 K. The obtained value of the critical exponent alpha =0.12 in the ferroelectric phase (T < TC) was consistent with that predicted from the 3-d Ising model (alpha =0.13), while the obtained value of alpha =0.32 in the paraelectric phase (T > TC) was consistent with that predicted from the 2-d potts model (alpha =0.30). Some thermodynamic quantities such as the internal energy, the entropy and the free energy of beta-glycine were then predicted in terms of these extracted values of the critical exponents close to the phase transition temperature of TC. Our calculated values of the thermodynamic quantities are in good agreement with the observed data.

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